The concept of topology has changed our perspectives on how to understand basic material properties. It allows us to predict and realize topologically protected edge or surface electronic states, the nature of which is free from material details. This leads to peculiar quantum transport behaviors, such as the Quantum Spin Hall Effect and Quantum Anomalous Hall Effect. Understanding how to precisely manipulate topological phases, particularly above the liquid helium temperatures, will lay the foundation for novel device concepts such as the topotronics.
Magnetic topological insulators are materials where intrinsic magnetism couples strongly to the topological electronic states, giving rise to a versatile material platform where distinct topological phases can be realized and tuned. We will use MRSTEP to manipulate the nonequilibrium topological phases of magnetic topological insulators, specifically the (MnBi2Te4)m(Bi2Te3)n family. We will fabricate (MnBi2Te4)m(Bi2Te3)n superlattices with atomic precision via molecular beam epitaxy, and disentangle spectroscopic features corresponding to different layer thicknesses and terminations via microARPES. We will also employ time-resolved ARPES to induce nonequilibrium topological changes of the electronic structure. Ultimately, the combination of precise spatial control and nonequilibrium engineering can lead to the revelation and manipulation of a nonequilibrium quantum anomalous Hall insulator state.